All Intel 960 machine instructions are supported; Section 23.1 i960 Command-line Options for a discussion of selecting the instruction subset for a particular 960 architecture.
Some opcodes are processed beyond simply emitting a single corresponding instruction: callj, and Compare-and-Branch or Compare-and-Jump instructions with target displacements larger than 13 bits.
You can write callj to have the assembler or the linker determine the most appropriate form of subroutine call: call, bal, or calls. If the assembly source contains enough information--a .leafproc or .sysproc directive defining the operand--then as translates the callj; if not, it simply emits the callj, leaving it for the linker to resolve.
The 960 architectures provide combined Compare-and-Branch instructions that permit you to store the branch target in the lower 13 bits of the instruction word itself. However, if you specify a branch target far enough away that its address won't fit in 13 bits, the assembler can either issue an error, or convert your Compare-and-Branch instruction into separate instructions to do the compare and the branch.
Whether as gives an error or expands the instruction depends on two choices you can make: whether you use the -no-relax option, and whether you use a "Compare and Branch" instruction or a "Compare and Jump" instruction. The "Jump" instructions are always expanded if necessary; the "Branch" instructions are expanded when necessary unless you specify -no-relax--in which case as gives an error instead.
These are the Compare-and-Branch instructions, their "Jump" variants, and the instruction pairs they may expand into: